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Abstract A new method that automatically determines the modality of an observed particle size distribution (PSD) and the representation of each mode as a gamma function was used to characterize data obtained during the High Altitude Ice Crystals and High Ice Water Content (HAIC-HIWC) project based out of Cayenne, French Guiana, in 2015. PSDs measured by a 2D stereo probe and a precipitation imaging probe for particles with maximum dimension ( D max ) > 55 μ m were used to show how the gamma parameters varied with environmental conditions, including temperature ( T ) and convective properties such as cloud type, mesoscale convective system (MCS) age, distance away from the nearest convective peak, and underlying surface characteristics. Four kinds of modality PSDs were observed: unimodal PSDs and three types of multimodal PSDs (Bimodal1 with breakpoints 100 ± 20 μ m between modes, Bimodal2 with breakpoints 1000 ± 300 μ m, and Trimodal PSDs with two breakpoints). The T and ice water content (IWC) are the most important factors influencing the modality of PSDs, with the frequency of multimodal PSDs increasing with increasing T and IWC. An ellipsoid of equally plausible solutions in ( N o – λ–μ ) phase space is defined for each mode of the observed PSDs for different environmental conditions. The percentage overlap between ellipsoids was used to quantify the differences between overlapping ellipsoids for varying conditions. The volumes of the ellipsoid decrease with increasing IWC for most cases, and ( N o – λ–μ ) vary with environmental conditions related to distribution of IWC. HIWC regions are dominated by small irregular ice crystals and columns. The parameters ( N o – λ–μ ) in each mode exhibit mutual dependence. 

Abstract Total ice water content (IWC) derived from an isokinetic evaporator probe and ice crystal particle size distributions (PSDs) measured by a two-dimensional stereo probe and precipitation imaging probe installed on an aircraft during the 2014 European High Altitude Ice Crystals–North American High IWC field campaign (HAIC/HIWC) were used to characterize regions of high IWC consisting mainly of small ice crystals (HIWC_S) with IWC ≥ 1.0 g m⁻³and median mass diameter (MMD) < 0.5 mm. A novel fitting routine developed to automatically determine whether a unimodal, bimodal, or trimodal gamma distribution best fits a PSD was used to compare characteristics of HIWC_S and other PSDs (e.g., multimodality, gamma fit parameters) for HIWC_S simulations. The variation of these characteristics and bulk properties (MMD, IWC) was regressed with temperature, IWC, and vertical velocity. HIWC_S regions were most pronounced in updraft cores. The three modes of the PSD reveal different dominant processes contributing to ice growth: nucleation for maximum dimensionD< 0.15 mm, diffusion for 0.15 <D< 1.0 mm, and aggregation forD> 1.0 mm. The frequency of trimodal distributions increased with temperature. The volumes of equally plausible parameters derived in the phase space of gamma fit parameters increased with temperature for unimodal distributions and, for temperatures less than −27°C, for multimodal distributions. Bimodal distributions with 0.4 mm in the larger mode were most common in updraft cores and HIWC_S regions; bimodal distributions with 0.4 mm in the smaller mode were least common in convective cores.